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Creators/Authors contains: "Strempfer, J"

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  1. Abstract Geometrically frustrated kagome lattices are raising as novel platforms to engineer correlated topological electron flat bands that are prominent to electronic instabilities. Here, we demonstrate a phonon softening at thekz = πplane in ScV6Sn6. The low energy longitudinal phonon collapses at ~98 K andq = $$\frac{1}{3}\frac{1}{3}\frac{1}{2}$$ 1 3 1 3 1 2 due to the electron-phonon interaction, without the emergence of long-range charge order which sets in at a different propagation vectorqCDW = $$\frac{1}{3}\frac{1}{3}\frac{1}{3}$$ 1 3 1 3 1 3 . Theoretical calculations corroborate the experimental finding to indicate that the leading instability is located at$$\frac{1}{3}\frac{1}{3}\frac{1}{2}$$ 1 3 1 3 1 2 of a rather flat mode. We relate the phonon renormalization to the orbital-resolved susceptibility of the trigonal Sn atoms and explain the approximately flat phonon dispersion. Our data report the first example of the collapse of a kagome bosonic mode and promote the 166 compounds of kagomes as primary candidates to explore correlated flat phonon-topological flat electron physics. 
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